The O-Directed Free Radical Hydrostannation of Propargyloxy Dialkyl Acetylenes with Ph<sub>3</sub> SnH/cat. Et<sub>3</sub> B. A Refutal of the Stannylvinyl Cation Mechanism.

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作者： Karl J,Hale ^[1] ; Soraya,Manaviazar ^[1] ; Hamish A,Watson ^[1]

作者单位： School of Chemistry and Chemical Engineering and the Centre for Cancer Research and Cell Biology (CCRCB), Queen's University Belfast, Stranmillis Road, Belfast, BT9 5AG, Northern Ireland, United Kingdom. ^[1]

关键词 Allylic 1,3-strain and 1,2-strain Internal Ligand Enhanced Radicalophilicity O-Directed Free Radical Hydrostannation with Ph3SnH/cat. Et3B Ph3Sn radicals have higher electron affinity Propargylically-Oxygenated Alkyl Acetylenes Stannylvinyl Radical The magnitudes of polar solvent rate accelerations observed for genuinely ionic reaction mechanisms Trisubstituted Stannylvinyl Radical H-Atom Abstraction Vinylperoxy radical Vinylstannane isomerisation β-Stannylvinyl cation

DOI 10.1002/tcr.201700104

PMID 30411498

发布时间 2019-11-20

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Chemical record (New York, N.Y.)

2019年19卷2-3期

238-319页

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The O-Directed Free Radical Hydrostannation of Propargyloxy Dialkyl Acetylenes with Ph<sub>3</sub> SnH/cat. Et<sub>3</sub> B. A Refutal of the Stannylvinyl Cation Mechanism.

Chemical record (New York, N.Y.)

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The O-Directed Free Radical Hydrostannation of Propargyloxy Dialkyl Acetylenes with Ph<sub>3</sub> SnH/cat. Et<sub>3</sub> B. A Refutal of the Stannylvinyl Cation Mechanism.

Chemical record (New York, N.Y.)

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Chemical record (New York, N.Y.)

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